Libra Compatibility Most Least Compatible SignsLibra love most suitable zodiac signs are twins, aquarius, and ram. When it comes to matters of the heart, Libra seeks harmony and compatibility above all else. Gemini can offer adventure and fun to the bond, while The Water Bearer shares Libra's appreciation for wisdom and innovation. The Ram, known for their passion, can ignite a desire in Libra's being. Libra and these signs create a well-rounded and satisfying partnership.